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The solubility of calcium carbonate in green liquor handling systems, TAPPI Journal October 2019

ABSTRACT: The formation of hard calcite (CaCO3) scale in green liquor handling systems is a persistent problem in many kraft pulp mills. CaCO3 precipitates when its concentration in the green liquor exceeds its solubility. While the solubility of CaCO3 in water is well known, it is not so in the highly alkaline green liquor environment. A systematic study was conducted to determine the solubility of CaCO3 in green liquor as a function of temperature, total titratable alkali (TTA), causticity, and sulfidity. The results show that the solubility increases with increased temperature, increased TTA, decreased causticity, and decreased sulfidity. The new solubility data was incorporated into OLI (a thermodynamic simulation program for aqueous salt systems) to generate a series of CaCO3 solubility curves for various green liquor conditions. The results help explain how calcite scale forms in green liquor handling systems.

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Guest Editorial: Recognizing excellence in recycling, TAPPI

Guest Editorial: Recognizing excellence in recycling, TAPPI JOURNAL February 2012

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Open Access
Importance of specimen preparation for edgewise compressive strength (ECT) testing, TAPPI JOURNAL April 2018

Importance of specimen preparation for edgewise compressive strength (ECT) testing, TAPPI JOURNAL April 2018

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Open Access
Editorial: Douglas Coffin: Paper Physics Guru, TAPPI JOURNAL August 2018

Editorial: Douglas Coffin: Paper Physics Guru, TAPPI JOURNAL August 2018

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Open Access
Prediction of box failure from paper data for asymmetric corrugated board, TAPPI JOURNAL August 2018

Prediction of box failure from paper data for asymmetric corrugated board, TAPPI JOURNAL August 2018

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Open Access
Impact of fiber structure on edge-wicking of highly-sized paperboard, TAPPI JOURNAL August 2018

Impact of fiber structure on edge-wicking of highly-sized paperboard, TAPPI JOURNAL August 2018

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Open Access
Editor's Note: Great expectations, TAPPI JOURNAL January 201

Editor's Note: Great expectations, TAPPI JOURNAL January 2011

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Open Access
Novel CaCO3-polymer nanocomposite fillers for the improvemen

Novel CaCO3-polymer nanocomposite fillers for the improvement of bagasse-based papers, November 2016 TAPPI JOURNAL

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Open Access
Combustion behavior of kraft black liquor droplets from hot

Combustion behavior of kraft black liquor droplets from hot water pretreated hardwood and softwood chips, November 2016 TAPPI JOURNAL

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Open Access
Static and dynamic sorption of lignin removed Populus euramericana, TAPPI JOURNAL February 2018

Static and dynamic sorption of lignin removed Populus euramericana, TAPPI JOURNAL February 2018

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